The fine spectral tuning of plasmon mode and quantum emitter coupling and its comparison with the dark-hot resonances

Authors: HIRA ASIF, RASİM VOLGA OVALI, RAMAZAN ŞAHİN

Abstract: Localization of incident fields into very small volumes (hot-spots) allows strong light-matter interactions at the hot spots. This makes path interference effects, Fano resonances, visible. Fano resonances can appear due to the coupling of a bright plasmon (i) to a longer lifetime dark plasmon mode or (ii) to a quantum object (QO) of a much longer lifetime. The second phenomenon provides a very important utility: the voltage tunability of the linear/nonlinear response. The level-spacing of the QO, such as defect-centers and quantum dots, are voltage-tunable which can make a sharp Fano resonance appear and disappear. Here, we compare the two phenomena by solving the equations of motions for the near-field plasmon amplitudes, derived from two different Hamiltonians. While the two plasmon amplitudes look similar to each other, except for the population inversion parameter `$y$', our results show that quantum emitter enables fine spectral tuning of the plasmon amplitude, thus, providing better enhancement.

Keywords: Localized surface plasmon (LSP), long-lived oscillators, bright and dark plasmon modes, fine-tuning response

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